Selectable Microporous Carbons Derived from Poplar Wood by Three Preparation Routes for CO2 Capture.
Identifieur interne : 000129 ( Main/Exploration ); précédent : 000128; suivant : 000130Selectable Microporous Carbons Derived from Poplar Wood by Three Preparation Routes for CO2 Capture.
Auteurs : Lishu Shao [République populaire de Chine] ; Yafei Sang [République populaire de Chine] ; Na Liu [République populaire de Chine] ; Jun Liu [République populaire de Chine] ; Peng Zhan [République populaire de Chine] ; Jianhan Huang [République populaire de Chine] ; Jienan Chen [République populaire de Chine]Source :
- ACS omega [ 2470-1343 ] ; 2020.
Abstract
Biomass-derived porous carbons are one kind of sustainable, extensive, and flexible carbon material for CO2 capture. Here, we prepared several microporous carbons from poplar wood by three preparation routes. Especially, the residues of the poplar wood after the bioethanol process were explored as precursors to prepare activated carbon by KOH and ZnCl2 activation. By the adjustment of the preparation routes and the optimization of the activation conditions, these porous carbons exhibited diversified morphology (sponge, nanosheets, and honeycomb structure), tunable porosity (specific surface areas: 511-2153 m2/g), and narrow micropore distribution (0.55-1.2 nm). These carbons had a high CO2 uptake of up to 217 mg/g at 273 K and 1 bar, which was comparable with those of many N-doped porous carbons, and possessed moderate isosteric heat of CO2 adsorption (21.1-43.2 kJ/mol), good cyclic ability, and high CO2/N2 selectivity (Henry's law: 44.0). The results indicated that CO2 uptake of these carbons was mainly decided by their micropore volume (d < 1.0 nm) at 273 K and 1 bar. This work provides an important reference for preparing promising CO2 adsorbents with tunable structures from similar biomass resources.
DOI: 10.1021/acsomega.0c01918
PubMed: 32715230
PubMed Central: PMC7377076
Affiliations:
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410004</wicri:regionArea><wicri:noRegion>Changsha 410004</wicri:noRegion></affiliation></author><author><name sortKey="Sang, Yafei" sort="Sang, Yafei" uniqKey="Sang Y" first="Yafei" last="Sang">Yafei Sang</name><affiliation wicri:level="1"><nlm:affiliation>College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Chemistry and Chemical Engineering, Central South University, Changsha 410083</wicri:regionArea><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name sortKey="Liu, Na" sort="Liu, Na" uniqKey="Liu N" first="Na" last="Liu">Na Liu</name><affiliation wicri:level="1"><nlm:affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004</wicri:regionArea><wicri:noRegion>Changsha 410004</wicri:noRegion></affiliation></author><author><name sortKey="Liu, Jun" sort="Liu, Jun" uniqKey="Liu J" first="Jun" last="Liu">Jun Liu</name><affiliation wicri:level="1"><nlm:affiliation>College of Resources and Environment, Hunan Agricultural University, Changsha 410128, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Resources and Environment, Hunan Agricultural University, Changsha 410128</wicri:regionArea><wicri:noRegion>Changsha 410128</wicri:noRegion></affiliation></author><author><name sortKey="Zhan, Peng" sort="Zhan, Peng" uniqKey="Zhan P" first="Peng" last="Zhan">Peng Zhan</name><affiliation wicri:level="1"><nlm:affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004</wicri:regionArea><wicri:noRegion>Changsha 410004</wicri:noRegion></affiliation></author><author><name sortKey="Huang, Jianhan" sort="Huang, Jianhan" uniqKey="Huang J" first="Jianhan" last="Huang">Jianhan Huang</name><affiliation wicri:level="1"><nlm:affiliation>College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Chemistry and Chemical Engineering, Central South University, Changsha 410083</wicri:regionArea><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name sortKey="Chen, Jienan" sort="Chen, Jienan" uniqKey="Chen J" first="Jienan" last="Chen">Jienan Chen</name><affiliation wicri:level="1"><nlm:affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004</wicri:regionArea><wicri:noRegion>Changsha 410004</wicri:noRegion></affiliation></author></analytic><series><title level="j">ACS omega</title><idno type="eISSN">2470-1343</idno><imprint><date when="2020" type="published">2020</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Biomass-derived porous carbons are one kind of sustainable, extensive, and flexible carbon material for CO<sub>2</sub> capture. Here, we prepared several microporous carbons from poplar wood by three preparation routes. Especially, the residues of the poplar wood after the bioethanol process were explored as precursors to prepare activated carbon by KOH and ZnCl<sub>2</sub> activation. By the adjustment of the preparation routes and the optimization of the activation conditions, these porous carbons exhibited diversified morphology (sponge, nanosheets, and honeycomb structure), tunable porosity (specific surface areas: 511-2153 m<sup>2</sup>/g), and narrow micropore distribution (0.55-1.2 nm). These carbons had a high CO<sub>2</sub> uptake of up to 217 mg/g at 273 K and 1 bar, which was comparable with those of many N-doped porous carbons, and possessed moderate isosteric heat of CO<sub>2</sub> adsorption (21.1-43.2 kJ/mol), good cyclic ability, and high CO<sub>2</sub>/N<sub>2</sub> selectivity (Henry's law: 44.0). The results indicated that CO<sub>2</sub> uptake of these carbons was mainly decided by their micropore volume (<i>d</i> < 1.0 nm) at 273 K and 1 bar. This work provides an important reference for preparing promising CO<sub>2</sub> adsorbents with tunable structures from similar biomass resources.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">32715230</PMID><DateRevised><Year>2020</Year><Month>09</Month><Day>28</Day></DateRevised><Article PubModel="Electronic-eCollection"><Journal><ISSN IssnType="Electronic">2470-1343</ISSN><JournalIssue CitedMedium="Internet"><Volume>5</Volume><Issue>28</Issue><PubDate><Year>2020</Year><Month>Jul</Month><Day>21</Day></PubDate></JournalIssue><Title>ACS omega</Title><ISOAbbreviation>ACS Omega</ISOAbbreviation></Journal><ArticleTitle>Selectable Microporous Carbons Derived from Poplar Wood by Three Preparation Routes for CO<sub>2</sub> Capture.</ArticleTitle><Pagination><MedlinePgn>17450-17462</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/acsomega.0c01918</ELocationID><Abstract><AbstractText>Biomass-derived porous carbons are one kind of sustainable, extensive, and flexible carbon material for CO<sub>2</sub> capture. Here, we prepared several microporous carbons from poplar wood by three preparation routes. Especially, the residues of the poplar wood after the bioethanol process were explored as precursors to prepare activated carbon by KOH and ZnCl<sub>2</sub> activation. By the adjustment of the preparation routes and the optimization of the activation conditions, these porous carbons exhibited diversified morphology (sponge, nanosheets, and honeycomb structure), tunable porosity (specific surface areas: 511-2153 m<sup>2</sup>/g), and narrow micropore distribution (0.55-1.2 nm). These carbons had a high CO<sub>2</sub> uptake of up to 217 mg/g at 273 K and 1 bar, which was comparable with those of many N-doped porous carbons, and possessed moderate isosteric heat of CO<sub>2</sub> adsorption (21.1-43.2 kJ/mol), good cyclic ability, and high CO<sub>2</sub>/N<sub>2</sub> selectivity (Henry's law: 44.0). The results indicated that CO<sub>2</sub> uptake of these carbons was mainly decided by their micropore volume (<i>d</i> < 1.0 nm) at 273 K and 1 bar. This work provides an important reference for preparing promising CO<sub>2</sub> adsorbents with tunable structures from similar biomass resources.</AbstractText><CopyrightInformation>Copyright © 2020 American Chemical Society.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Shao</LastName><ForeName>Lishu</ForeName><Initials>L</Initials><AffiliationInfo><Affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Sang</LastName><ForeName>Yafei</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Na</ForeName><Initials>N</Initials><AffiliationInfo><Affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Jun</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>College of Resources and Environment, Hunan Agricultural University, Changsha 410128, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhan</LastName><ForeName>Peng</ForeName><Initials>P</Initials><AffiliationInfo><Affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Huang</LastName><ForeName>Jianhan</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Chen</LastName><ForeName>Jienan</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>Ministry of Forestry Bioethanol Research Center, School of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2020</Year><Month>07</Month><Day>10</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Omega</MedlineTA><NlmUniqueID>101691658</NlmUniqueID><ISSNLinking>2470-1343</ISSNLinking></MedlineJournalInfo><CoiStatement>The authors declare no competing financial interest.</CoiStatement></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2020</Year><Month>04</Month><Day>25</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2020</Year><Month>06</Month><Day>26</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2020</Year><Month>7</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2020</Year><Month>7</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2020</Year><Month>7</Month><Day>28</Day><Hour>6</Hour><Minute>1</Minute></PubMedPubDate></History><PublicationStatus>epublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">32715230</ArticleId><ArticleId 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sort="Shao, Lishu" uniqKey="Shao L" first="Lishu" last="Shao">Lishu Shao</name></noRegion><name sortKey="Chen, Jienan" sort="Chen, Jienan" uniqKey="Chen J" first="Jienan" last="Chen">Jienan Chen</name><name sortKey="Huang, Jianhan" sort="Huang, Jianhan" uniqKey="Huang J" first="Jianhan" last="Huang">Jianhan Huang</name><name sortKey="Liu, Jun" sort="Liu, Jun" uniqKey="Liu J" first="Jun" last="Liu">Jun Liu</name><name sortKey="Liu, Na" sort="Liu, Na" uniqKey="Liu N" first="Na" last="Liu">Na Liu</name><name sortKey="Sang, Yafei" sort="Sang, Yafei" uniqKey="Sang Y" first="Yafei" last="Sang">Yafei Sang</name><name sortKey="Zhan, Peng" sort="Zhan, Peng" uniqKey="Zhan P" first="Peng" last="Zhan">Peng Zhan</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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